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Biomimmetic Catalytic Asymmetric Synthesis of the Bisorbicillinoids and Related Products PhD
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Biomimmetic Catalytic Asymmetric Synthesis of the Bisorbicillinoids and Related Products PhD
Loughborough University, Loughborough, United Kingdom
# 301-350QS Subject Rankings
36 monthsProgram duration
27,500 Tuition Fee/year
01 Apr, 2025Application Deadline
Program overview
Main Subject
Chemistry
Degree
PhD
Study Level
PHD
Study Mode
On Campus
Read more Our approach utilises the new application of a catalyst that is only comprised of organic components - know as an organocatalyst. Organocatalysis is a particularly topical area since the 2021 Nobel Prize for chemistry was awarded to Prof. D. Macmillan and Prof. B. List for their ground breaking work in establishing the field in the early 2000's.
The dearomatisation of stable aromatic building blocks provides rapid routes to often complex natural product frameworks. However, the selective construction of such compounds in a catalytic highly enantioselective fashion remains a long-standing challenge. It is only recently that our group reported preliminary studies on a highly enantioselective organocatalytic route to hydroxylative dearomatisation, exemplified in the synthesis of (+)-biscaravacrol in 61% yield and 99:1 e.r. in one synthetic step from carvacrol. Please see related online paper.
We will develop a novel highly enantioselective route to previously difficult to access natural and non-natural products. This new methodology will give practical access to gram quantities of known bisorbicillinoids and new non-natural analogues which we believe will be a valuable class of compounds for future investigators interested in the biological activity of small molecules. Given our preliminary results and experience with oxaziridinium catalysed processes we are confident that we can successfully achieve the aims and objectives of this proposal. Read less
Program overview
Main Subject
Chemistry
Degree
PhD
Study Level
PHD
Study Mode
On Campus
Read more Our approach utilises the new application of a catalyst that is only comprised of organic components - know as an organocatalyst. Organocatalysis is a particularly topical area since the 2021 Nobel Prize for chemistry was awarded to Prof. D. Macmillan and Prof. B. List for their ground breaking work in establishing the field in the early 2000's.
The dearomatisation of stable aromatic building blocks provides rapid routes to often complex natural product frameworks. However, the selective construction of such compounds in a catalytic highly enantioselective fashion remains a long-standing challenge. It is only recently that our group reported preliminary studies on a highly enantioselective organocatalytic route to hydroxylative dearomatisation, exemplified in the synthesis of (+)-biscaravacrol in 61% yield and 99:1 e.r. in one synthetic step from carvacrol. Please see related online paper.
We will develop a novel highly enantioselective route to previously difficult to access natural and non-natural products. This new methodology will give practical access to gram quantities of known bisorbicillinoids and new non-natural analogues which we believe will be a valuable class of compounds for future investigators interested in the biological activity of small molecules. Given our preliminary results and experience with oxaziridinium catalysed processes we are confident that we can successfully achieve the aims and objectives of this proposal. Read less
Admission Requirements
Tuition Fee and Scholarships
Domestic Students
International Students
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QS subject rankings
Subject: Chemistry
Ranking criteria
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Communication and Social Change (CSC) Hub Studentship PhD
Communication and Social Change (CSC) Hub Studentship PhD
Enhancing Motivation in Sport and Exercise Contexts PhD
Enhancing Motivation in Sport and Exercise Contexts PhD
Out of School Youth Provision: An Analysis of Funding and Operational Resilience within the Sector PhD
Out of School Youth Provision: An Analysis of Funding and Operational Resilience within the Sector PhD